Dr. Yimu Chen has made
transformative impacts on single-crystal hybrid halide perovskites and can
fundamentally accelerate the industrialization of this emerging class of semiconductor
materials.
Halide perovskites have
received extensive attention because of their exceptional optoelectronic
properties and device performance. While most studies focus on polycrystalline
halide perovskites due to the fabrication simplicity, single-crystal halide perovskites
hold a bright future in commercialization owing to the reduced defects,
enhanced stability and reliability, and the potential to break the performance
limit. Currently, single-crystal halide perovskite devices are becoming one of
the most mainstream in the field.
In the semiconductor
industry, epitaxial growth is one of the main approaches to obtain high-quality
single-crystal materials. The single-crystal epitaxial growth of complex
compounds such as halide perovskite epitaxy is one of the most difficult topics
in epitaxial growth technology.
Strain engineering has been
one of the most successful and widely-used techniques in the semiconductor
industry to boost the performance of semiconductor devices. While the novel
semiconductor halide perovskites have been widely studied, controllable strain
engineering of halide perovskites has not been systematically demonstrated due
to the relatively weak interfacial interaction at the epitaxial interface. Dr.
Chen achieved the first controllable strain engineering of the halide
perovskites based on the epitaxial halide perovskite thin films, demonstrating
the controllable strain engineering and the epitaxial stabilization effect in
the epitaxial halide perovskites.
Dr. Chen has developed a
novel fabrication method for high-performance single-crystal halide perovskite
devices, including a transfer method of the single-crystal halide perovskite
thin film for device integration.
Solving the incompatibility
between halide perovskites and semiconductor nano/microfabrication, Dr. Chen
has demonstrated the first halide perovskite single-crystal micro-LEDs. Aiming
at solving this incompatibility, he designs a dense polymer parylene-C
protection layer as extra protection to the halide perovskite single crystals
so that halide perovskite single crystals are free from the damage by moisture during the photolithography and the wet etching process.